Alfred

-The ever-faithful Alfred Pennyworth! Give him a feather-duster and his green apron, and, boom, we're good to go. As big a role as this version of Alfred played on the show--fist-fighting the likes of Penguin and Joker!--he deserves the Pop treatment!
Alfred as Batman

This one's a no-brainer! Alfred dressed up as Batman in several episodes. And the characters always fell for it! Would LOVE to see this one.
Batgirl & Batgirl Cycle

Her Cycle is one of the most iconic aspects of the Series! We need to be able to put it with the Batmobile!
Bookworm

While he only appeared in two episodes, Bookworm is actually one of the Series' BEST villains! And his design would lend itself well to a Pop! If you haven't seen his two-parter, check it out!
Boxing Batman
Boxing Riddler

How about a two-pack? From the episode Ring Around the Riddler, this, for me, is every bit as iconic as Surf's Up, Joker's Under.
Catwoman (Unmasked)

We NEED to get Julie Newmar's incredible and iconic eyebrows on a figure! Plus, she spent more time UNMASKED than MASKED!
Catwoman (Eartha Kitt)

-Obviously.
Catwoman Goon

I think these henchmen have such iconic designs, we need them to put with the Baddies!
Contaminated Cowl Batman

From the Mad Hatter episode of the same name, a cool variant. Just repaint his cowl pink! Easy money, Funko!
Egghead

EGGSellent! This EGGStraordinary villain is just too EGGciting to pass up! Vincent Price and egg-puns! C'mon! (This is actually my most-wanted figure of the line currently,

The Joker-Mobile

Joker's famous Jokermobile would make an awesome Ride!
The Mad Hatter

This guy got four episodes and is all ready one of the most iconic Batman rogues. I always thought the '66 version was the nastiest and most wicked of the Mad Hatters!
Mr. Freeze (Eli Wallach)
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UGH. It pains me to see so much Otto Preminger Mr. Freeze merch when Wallach's take is so much more enjoyable! I want THIS Freeze, not the one with the orange eyebrows (Preminger's annoying habit of saying, "WILD!" every sentence really irritates me. It helps to know that Preminger was apparently a major jerk on the set of the show, disliked by the cast). Wallach for the win!
Penguin Goons

Again, ICONIC henchmen. We need one!
The Riddler (John Astin)

John Astin's Riddler. It's a shame Gorshin didn't perform for this two-parter, because, in my opinion, it's actually the best-WRITTEN Riddler story in the show's run. It just has a lackluster Riddler... Nevertheless, Astin IS a part of the show's history and therefore, I think we need an Astin Riddler (holding his question-mark cane!)
TWO-FACE

Even though he's only just about to make his animated debut into the Batman '66 world, I think William Shatner's Two-Face, with his amazing Golden-Age inspired design, would make a FINE Pop and would fit right in with the rest!